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A Delicately Designed Sulfide Graphdiyne Compatible Cathode for High-Performance Lithium/Magnesium-Sulfur Batteries
Du Huiping; Zhang Zhonghua; He Jianjiang; Cui Zili; Chai Jingchao; Ma Jun; Yang Ze; Huang Changshui; Cui Guanglei
2017-09-28
Source PublicationSmall
Volume13Issue:44Pages:1702277
AbstractNovel sulfur cathodes hold the key to the development of metal-sulfur batteries, the promising candidate of next-generation high-energy-storage systems. Herein, a fascinating sulfur cathode based on sulfide graphdiyne (SGDY) is designed with a unique structure, which is composed of a conducting carbon skeleton with high Li+ mobility and short sulfur energy-storing unites. The SGDY cathode can essentially avoid polysulfide dissolution and be compatible with commercially available carbonate-based electrolytes and Grignard reagent-based electrolytes (all phenyl complex (APC) type electrolytes). Both the assembled Li-S and Mg-S batteries exhibit excellent electrochemical performances including large capacity, superior rate capability, high capacity retention, and high Coulombic efficiency. More importantly, this is the first implementation case of a reliable Mg-S system based on nucleophilic APC electrolytes.
SubtypeArticle
WOS HeadingsChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
DOI10.1002/smll.201702277
WOS KeywordLI-S BATTERIES ; LITHIUM STORAGE ; POROUS CARBON ; CYCLING STABILITY ; GRAPHENE OXIDE ; POLYSULFIDE ; ELECTROLYTE ; CAPACITY ; NITROGEN ; RAMAN
Indexed BySCI
Language英语
WOS Research AreaChemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
Funding OrganizationQingdao Key Lab of Solar Energy Utilization and Energy Storage Technology National Natural Science Foundation of China 21271180 Key Technology Research Projects of Qingdao 13-CX-10
WOS SubjectChemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS IDWOS:000416040600009
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Document Type期刊论文
Identifierhttp://ir.qibebt.ac.cn/handle/337004/9886
Collection新型能源碳素材料团队
Affiliation1.中国科学院青岛生物能源与过程研究所
2.中国科学院大学
Recommended Citation
GB/T 7714
Du Huiping,Zhang Zhonghua,He Jianjiang,et al. A Delicately Designed Sulfide Graphdiyne Compatible Cathode for High-Performance Lithium/Magnesium-Sulfur Batteries[J]. Small,2017,13(44):1702277.
APA Du Huiping.,Zhang Zhonghua.,He Jianjiang.,Cui Zili.,Chai Jingchao.,...&Cui Guanglei.(2017).A Delicately Designed Sulfide Graphdiyne Compatible Cathode for High-Performance Lithium/Magnesium-Sulfur Batteries.Small,13(44),1702277.
MLA Du Huiping,et al."A Delicately Designed Sulfide Graphdiyne Compatible Cathode for High-Performance Lithium/Magnesium-Sulfur Batteries".Small 13.44(2017):1702277.
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