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Acceptor-rich bulk heterojunction polymer solar cells with balanced charge mobilities
Zhu, Tingting1,2; Zhang, Yongchao1; Li, Yonghai1; Song, Xin2; Liu, Zhe2; Wen, Shuguang1; Bao, Xichang1; Sun, Mingliang2; Yang, Renqiang1
2017-12-01
发表期刊ORGANIC ELECTRONICS
卷号51页码:16-24
摘要In this work, we reported efficient polymer solar cells with balanced hole/electron mobilities tuned by the acceptor content in bulk heterojunction blend films. The photovoltaic cells were fabricated with two new wide band-gap D-A polymers PBDDIDT and PBDDIDTT as the donor material. The molecular conformations of new polymers are carefully evaluated by theoretical calculations. The results of photovoltaic studies show that two devices reach their optimal conditions with rich PC71BM content up to 80% in blend films, which is uncommon with most of reported PSCs. The as-cast devices based on PBDDIDT and PBDDIDTT reveal good photovoltaic performance with PCE of 7.04% and 6.40%, respectively. The influence of PC71BM content on photovoltaic properties is further detailed studied by photoluminescence emission spectra, charge mobilities and heterojunction morphology. The results exhibit that more efficient charge transport between donor and acceptor occurs in rich PC71BM blend films. Meanwhile, the hole and electron mobilities are simultaneously enhanced and afford a good balance in rich PC71BM blend films (D/A, 1: 4) which is critical for the improvement of current density and fill factors. (C) 2017 Elsevier B.V. All rights reserved.
文章类型Article
关键词Wide Band-gap Acceptor-rich Blend Polymer Solar Cells Balanced Charge Mobilities
WOS标题词Science & Technology ; Technology ; Physical Sciences
DOI10.1016/j.orgel.2017.08.031
关键词[WOS]POWER CONVERSION EFFICIENCY ; SMALL-MOLECULE ACCEPTOR ; OPEN-CIRCUIT VOLTAGE ; HIGH-PERFORMANCE ; CONJUGATED POLYMER ; PHOTOVOLTAIC PERFORMANCE ; ELECTRON-ACCEPTORS ; ALKYL CHAINS ; DONOR ; COPOLYMERS
收录类别SCI
语种英语
WOS研究方向Materials Science ; Physics
项目资助者National Natural Science Foundation of China(21502205 ; Ministry of Science and Technology of China(2016YFE0115000) ; China Postdoctoral Science Foundation(2016T90656) ; 51573205)
WOS类目Materials Science, Multidisciplinary ; Physics, Applied
WOS记录号WOS:000418101600004
引用统计
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/9825
专题先进有机功能材料团队
作者单位1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, CAS Key Lab Biobased Mat, Qingdao 266101, Peoples R China
2.Ocean Univ China, Inst Mat Sci & Engn, Qingdao 266100, Peoples R China
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Zhu, Tingting,Zhang, Yongchao,Li, Yonghai,et al. Acceptor-rich bulk heterojunction polymer solar cells with balanced charge mobilities[J]. ORGANIC ELECTRONICS,2017,51:16-24.
APA Zhu, Tingting.,Zhang, Yongchao.,Li, Yonghai.,Song, Xin.,Liu, Zhe.,...&Yang, Renqiang.(2017).Acceptor-rich bulk heterojunction polymer solar cells with balanced charge mobilities.ORGANIC ELECTRONICS,51,16-24.
MLA Zhu, Tingting,et al."Acceptor-rich bulk heterojunction polymer solar cells with balanced charge mobilities".ORGANIC ELECTRONICS 51(2017):16-24.
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