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High-performance ternary polymer solar cells from a structurally similar polymer alloy
Shen, Wenfei1,2; Chen, Weichao1,2; Zhu, Dangqiang1; Zhang, Jidong4; Xu, Xiaofeng3; Jiang, Huanxiang1; Wang, Ting1; Wang, Ergang3; Yang, Renqiang1
2017-06-28
Source PublicationJOURNAL OF MATERIALS CHEMISTRY A
Volume5Issue:24Pages:12400-12406
AbstractHigh-efficiency ternary polymer solar cells (PSCs) are fabricated by using two donor polymers (PBDTTPD and PBDTTT-C-T) with similar polymer backbones and complementary absorption and PC71BM as the acceptor. A high power conversion efficiency (PCE) of 9.3% is achieved with a high short-circuit current density (J(sc)) of 17.2 mA cm(-2). The enhanced J(sc) and PCEs are mainly attributed to the broadened photoresponse of the ternary blend. Good miscibility of the two donor polymers is found due to the similar polymer main chains, leading to the desired morphology between the donors and PC71BM in the ternary blends. The trend of open-circuit voltage (V-oc) variations indicates the formation of a polymer alloy in this ternary blend. Our work demonstrates that using two donor polymers with similar backbone structures is a rational strategy for realizing high-performance ternary PSCs.
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1039/c7ta02891a
WOS KeywordPOWER CONVERSION EFFICIENCY ; 25TH ANNIVERSARY ARTICLE ; SMALL-MOLECULE ; NONFULLERENE ACCEPTORS ; 11-PERCENT EFFICIENCY ; IR SENSITIZATION ; ENERGY-TRANSFER ; FULLERENE ; CHAINS
Indexed BySCI
Language英语
WOS Research AreaChemistry ; Energy & Fuels ; Materials Science
Funding OrganizationNational Natural Science Foundation of China(61405209 ; Ministry of Science and Technology of China(2014CB643501 ; 51573205 ; 2010DFA52310) ; 21604092)
WOS SubjectChemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary
WOS IDWOS:000403664800047
Citation statistics
Document Type期刊论文
Identifierhttp://ir.qibebt.ac.cn/handle/337004/9651
Collection先进有机功能材料研究组
Affiliation1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, CAS Key Lab Biobased Mat, Qingdao 266101, Peoples R China
2.Qingdao Univ, Coll Text & Clothing, Qingdao 266071, Peoples R China
3.Chalmers, Dept Chem & Chem Engn Polymer Technol, SE-41296 Gothenburg, Sweden
4.Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Polymer Phys & Chem, Changchun 130022, Peoples R China
Recommended Citation
GB/T 7714
Shen, Wenfei,Chen, Weichao,Zhu, Dangqiang,et al. High-performance ternary polymer solar cells from a structurally similar polymer alloy[J]. JOURNAL OF MATERIALS CHEMISTRY A,2017,5(24):12400-12406.
APA Shen, Wenfei.,Chen, Weichao.,Zhu, Dangqiang.,Zhang, Jidong.,Xu, Xiaofeng.,...&Yang, Renqiang.(2017).High-performance ternary polymer solar cells from a structurally similar polymer alloy.JOURNAL OF MATERIALS CHEMISTRY A,5(24),12400-12406.
MLA Shen, Wenfei,et al."High-performance ternary polymer solar cells from a structurally similar polymer alloy".JOURNAL OF MATERIALS CHEMISTRY A 5.24(2017):12400-12406.
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