QIBEBT-IR  > 膜分离与催化团队
Syngas Production by Biogas Reforming in a Redox-Stable and CO2-Tolerant Oxygen Transporting Membrane Reactor
He, Guanghu1; Hu, Tianmiao1,2; Zhou, Hangyue1,2; Liang, Fangyi1; Baumann, Stefan3; Meulenberg, Wilhelm A.3; Jiang, Heqing1
2017-09-13
发表期刊INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
卷号56期号:36页码:10134-10141
摘要A novel membrane reactor consisting of Ce0.9Gd0.1O2-delta Gd0.1Sr0.9Fe0.9Ti0.1O3-delta (CGOGSFT) is used to combine air separation with biogas reforming in a single unit. The composite material CGOGSFT was synthesized via a combined EDTAcitrate complexing solgel method. Characterization with XRD, SEM, and EDXS revealed that the composite material was a two-phase fluoriteperovskite system with good compatibility and a homogeneous percolative network. XRD demonstrated that the CGOGSFT membrane shows a good phase stability not only in CO2 but also in simulated biogas atmosphere. Under the gradient of air/simulated biogas, the oxygen permeability and methane conversion was increased by either raising the operating temperature or increasing the CO2 concentration. At 890 degrees C and a CH4/CO2 molar ratio of 1.5, an oxygen permeation flux of 1.1 cm(3) min(1) cm(2) through the CGOGSFT membrane was achieved while methane conversion reached 83%, and remained stable for nearly 150 h before the measurement was intentionally stopped.
文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1021/acs.iecr.7b01422
关键词[WOS]DUAL-PHASE MEMBRANE ; HOLLOW-FIBER MEMBRANES ; PEROVSKITE MEMBRANES ; COBALT-FREE ; HYDROGEN-PRODUCTION ; COMPOSITE MEMBRANE ; METHANE CONVERSION ; PERMEABLE MEMBRANE ; CERAMIC MEMBRANES ; PARTIAL OXIDATION
收录类别SCI
语种英语
WOS研究方向Engineering
项目资助者National Natural Science Foundation of China(21506237 ; Shandong Provincial Natural Science Foundation, China(BS201SNJ002) ; China Postdoctoral Science Foundation(2015M570617) ; State Key Laboratory of Coal Conversion(J15-16-907) ; project of the Science and Technology Development Program in Shandong Province(2014GSF117031) ; 21471156)
WOS类目Engineering, Chemical
WOS记录号WOS:000411043700022
引用统计
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/9580
专题膜分离与催化团队
作者单位1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao Key Lab Funct Membrane Mat & Membrane Tec, Qingdao 266101, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Forschungszentrum Julich, Inst Energy & Climate Res IEK 1, D-52425 Julich, Germany
推荐引用方式
GB/T 7714
He, Guanghu,Hu, Tianmiao,Zhou, Hangyue,et al. Syngas Production by Biogas Reforming in a Redox-Stable and CO2-Tolerant Oxygen Transporting Membrane Reactor[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2017,56(36):10134-10141.
APA He, Guanghu.,Hu, Tianmiao.,Zhou, Hangyue.,Liang, Fangyi.,Baumann, Stefan.,...&Jiang, Heqing.(2017).Syngas Production by Biogas Reforming in a Redox-Stable and CO2-Tolerant Oxygen Transporting Membrane Reactor.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,56(36),10134-10141.
MLA He, Guanghu,et al."Syngas Production by Biogas Reforming in a Redox-Stable and CO2-Tolerant Oxygen Transporting Membrane Reactor".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 56.36(2017):10134-10141.
条目包含的文件
条目无相关文件。
个性服务
推荐该条目
保存到收藏夹
查看访问统计
导出为Endnote文件
谷歌学术
谷歌学术中相似的文章
[He, Guanghu]的文章
[Hu, Tianmiao]的文章
[Zhou, Hangyue]的文章
百度学术
百度学术中相似的文章
[He, Guanghu]的文章
[Hu, Tianmiao]的文章
[Zhou, Hangyue]的文章
必应学术
必应学术中相似的文章
[He, Guanghu]的文章
[Hu, Tianmiao]的文章
[Zhou, Hangyue]的文章
相关权益政策
暂无数据
收藏/分享
所有评论 (0)
暂无评论
 

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。