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Synergically Improving Light Harvesting and Charge Transportation of TiO2 Nanobelts by Deposition of MoS2 for Enhanced Photocatalytic Removal of Cr(VI)
Liu, Jie1; Li, Ying1; Ke, Jun2; Wang, Zhong3; Xiao, Huining1
2017
发表期刊CATALYSTS
卷号7期号:1
摘要Herein, MoS2/TiO2 nanobelts heterojunction have been successfully synthesized by in situ growth method for photocatalytic reduction of Cr(VI). TiO2 nanobelts (NBs) with rough surface were prepared firstly by acidic treatment process, which is beneficial for deposition and growth of MoS2 to form heterojunctions. As a result of special energy level offset and nanostructure, MoS2/TiO2 NBs composite were endowed with higher light-harvesting capacity and charge transportation efficiency, which are indispensible merits for excellent photocatalytic activity. The photocatalytic reduction of Cr(VI) reveals that the synthesized MoS2/TiO2 NBs composite have superior photocatalytic ability than other samples. Meanwhile, a photoreduction mechanism is proposed based on the systematic investigation, where the photogenerated electrons are demonstrated as the dominant reductive species to reduce Cr(VI) to Cr(III).
文章类型Article
关键词Environmental Remediation Cr(Vi) Photocatalysis Tio2 Nbs Mos2
WOS标题词Science & Technology ; Physical Sciences
DOI10.3390/catal7010030
关键词[WOS]HYDROGEN EVOLUTION ; H-2 EVOLUTION ; 101 FACETS ; PERFORMANCE ; REDUCTION ; NANOSTRUCTURES ; NANOSHEETS ; OXIDATION ; HETEROSTRUCTURES ; HETEROJUNCTION
收录类别SCI
语种英语
WOS研究方向Chemistry
项目资助者National Natural Science Foundation of China(21507029 ; Natural Science Foundation of Hubei Province(2015CFB177) ; China Ministry of Education ; Fundamental Research Funds for the Central Universities(2016MS109) ; Nature Science Foundation of Hebei Province(B2016502063) ; Open Foundation of Key Laboratory of Industrial Ecology and Environmental Engineering(KLIEEE-15-02) ; 21501138 ; 51379077)
WOS类目Chemistry, Physical
WOS记录号WOS:000395426100029
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文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/9324
专题多相催化转化研究组
作者单位1.North China Elect Power Univ, Sch Environm Sci & Engn, Baoding 071003, Peoples R China
2.Wuhan Inst Technol, Sch Chem & Environm Engn, Wuhan 430072, Peoples R China
3.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biofuels, Qingdao 266101, Peoples R China
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Liu, Jie,Li, Ying,Ke, Jun,et al. Synergically Improving Light Harvesting and Charge Transportation of TiO2 Nanobelts by Deposition of MoS2 for Enhanced Photocatalytic Removal of Cr(VI)[J]. CATALYSTS,2017,7(1).
APA Liu, Jie,Li, Ying,Ke, Jun,Wang, Zhong,&Xiao, Huining.(2017).Synergically Improving Light Harvesting and Charge Transportation of TiO2 Nanobelts by Deposition of MoS2 for Enhanced Photocatalytic Removal of Cr(VI).CATALYSTS,7(1).
MLA Liu, Jie,et al."Synergically Improving Light Harvesting and Charge Transportation of TiO2 Nanobelts by Deposition of MoS2 for Enhanced Photocatalytic Removal of Cr(VI)".CATALYSTS 7.1(2017).
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