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Highly Selective Upgrading of Biomass-Derived Alcohol Mixtures for Jet/Diesel-Fuel Components
Liu, Qiang1,2; Xu, Guoqiang1; Wang, Xicheng1; Liu, Xiaoran1,2; Mu, Xindong1
2016-12-20
发表期刊CHEMSUSCHEM
卷号9期号:24页码:3465-3472
摘要In light of the increasing concern about the energy and environmental problems caused by the combustion of petroleum-based fuels (e.g., jet and diesel fuels), the development of new procedures for their sustainable production from renewable biomass-derived platform compounds has attracted tremendous attention recently. Long-chain ketones/alcohols are promising fuel components owing to the fuel properties that closely resemble those of traditional fuels. The focus of this report is the production of long-chain ketones/alcohols by direct upgrading of biomass-derived short-chain alcohol mixtures (e.g., isopropanol-butanol-ethanol mixtures) in pure water. An efficient Pd catalyst system was developed for these highly selective transformations. Long-chain ketones/alcohols (C-8-C-19), which can be used as precursors for renewable jet/diesel fuel, were obtained in good-to-high selectivity (>90%) by using the developed Pd catalyst.
文章类型Article
关键词Alcohols Condensation Long-chain Oxygenates Palladium Supported Catalysts
WOS标题词Science & Technology ; Physical Sciences
DOI10.1002/cssc.201601152
关键词[WOS]N-DOPED CARBON ; ENGINEERING CLOSTRIDIUM-ACETOBUTYLICUM ; CATALYTIC CONVERSION ; TRANSPORTATION FUELS ; BORROWING HYDROGEN ; PALLADIUM CATALYST ; PLATFORM MOLECULES ; ESCHERICHIA-COLI ; ALPHA-ALKYLATION ; PD NANOPARTICLES
收录类别SCI
语种英语
WOS研究方向Chemistry
项目资助者Boeing(2014-JRLSAB-03) ; National Natural Science Foundation of China(21273260 ; Shandong Provincial Natural Science Foundation for Distinguished Young Scholar(JQ201305) ; Youth Innovation Promotion Association CAS(2015168) ; 21433001)
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000394571500015
引用统计
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/9320
专题绿色化学催化研究组
作者单位1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, CAS Key Lab Biobased Mat, Qingdao 266101, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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GB/T 7714
Liu, Qiang,Xu, Guoqiang,Wang, Xicheng,et al. Highly Selective Upgrading of Biomass-Derived Alcohol Mixtures for Jet/Diesel-Fuel Components[J]. CHEMSUSCHEM,2016,9(24):3465-3472.
APA Liu, Qiang,Xu, Guoqiang,Wang, Xicheng,Liu, Xiaoran,&Mu, Xindong.(2016).Highly Selective Upgrading of Biomass-Derived Alcohol Mixtures for Jet/Diesel-Fuel Components.CHEMSUSCHEM,9(24),3465-3472.
MLA Liu, Qiang,et al."Highly Selective Upgrading of Biomass-Derived Alcohol Mixtures for Jet/Diesel-Fuel Components".CHEMSUSCHEM 9.24(2016):3465-3472.
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