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Title:
A sustainable process for the production of 2-methyl-1,4-butanediol by hydrogenation of biomass-derived itaconic acid
Author: Liu, Xiaoran1,2; Wang, Xicheng1; Liu, Qiang1,2; Xu, Guoqiang1; Li, Xuemin1; Mu, Xindong1
Source: CATALYSIS TODAY
Issued Date: 2016-10-01
Volume: 274, Pages:88-93
Keyword: Biomass ; Itaconic acid ; 2-Methyl-1,4-Butanediol ; Hydrogenation ; Pd-ReOx/C
DOI: 10.1016/j.cattod.2016.01.041
DOC Type: Article
English Abstract: Pd-ReOx/C catalysts with different Re contents were prepared and employed to catalyze the aqueous hydrogenation of itaconic acid in this study. The Pd-ReOx/C catalysts were characterized by XRD, TEM, BET, NH3-TPD and H-2-TPR. Results showed that the addition of ReOx species in supported Pd catalysts promoted the direct conversion of itaconic acid to 2-methyl-1,4-butanediol. The promoting effect was ascribed to the interaction between Pd and ReOx species, as has been proved by the characterizations. A 2-methyl-1,4-butanediol yield of above 80% could be obtained over Pd-3ReO(x)/C under the reaction condition of 180 degrees C, 4 MPa H-2. (C) 2016 Elsevier B.V. All rights reserved.
WOS Headings: Science & Technology ; Physical Sciences ; Technology
WOS Subject: Chemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
WOS Subject Extended: Chemistry ; Engineering
WOS Keyword Plus: AQUEOUS-PHASE HYDROGENATION ; SUCCINIC ACID ; LIGNOCELLULOSIC BIOMASS ; GAMMA-BUTYROLACTONE ; PD/TIO2 CATALYSTS ; HYDROGENOLYSIS ; CHEMICALS ; PLATFORM ; CARBON ; TETRAHYDROFURAN
Indexed Type: SCI ; ISTP
Language: 英语
WOS ID: WOS:000377388300015
Citation statistics:
Content Type: 期刊论文
URI: http://ir.qibebt.ac.cn/handle/337004/8235
Appears in Collections:绿色化学催化团队_期刊论文

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description.institution: 1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biobased Mat, Qingdao 266101, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China

Recommended Citation:
Liu, Xiaoran,Wang, Xicheng,Liu, Qiang,et al. A sustainable process for the production of 2-methyl-1,4-butanediol by hydrogenation of biomass-derived itaconic acid[J]. CATALYSIS TODAY,2016,274:88-93.
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