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A sustainable process for the production of 2-methyl-1,4-butanediol by hydrogenation of biomass-derived itaconic acid
Liu, Xiaoran1,2; Wang, Xicheng1; Liu, Qiang1,2; Xu, Guoqiang1; Li, Xuemin1; Mu, Xindong1
2016-10-01
发表期刊CATALYSIS TODAY
卷号274页码:88-93
摘要Pd-ReOx/C catalysts with different Re contents were prepared and employed to catalyze the aqueous hydrogenation of itaconic acid in this study. The Pd-ReOx/C catalysts were characterized by XRD, TEM, BET, NH3-TPD and H-2-TPR. Results showed that the addition of ReOx species in supported Pd catalysts promoted the direct conversion of itaconic acid to 2-methyl-1,4-butanediol. The promoting effect was ascribed to the interaction between Pd and ReOx species, as has been proved by the characterizations. A 2-methyl-1,4-butanediol yield of above 80% could be obtained over Pd-3ReO(x)/C under the reaction condition of 180 degrees C, 4 MPa H-2. (C) 2016 Elsevier B.V. All rights reserved.
文章类型Article
关键词Biomass Itaconic Acid Hydrogenation 2-methyl-1 Pd-reox/c 4-butanediol
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.cattod.2016.01.041
关键词[WOS]AQUEOUS-PHASE HYDROGENATION ; SUCCINIC ACID ; LIGNOCELLULOSIC BIOMASS ; GAMMA-BUTYROLACTONE ; PD/TIO2 CATALYSTS ; HYDROGENOLYSIS ; CHEMICALS ; PLATFORM ; CARBON ; TETRAHYDROFURAN
收录类别SCI ; ISTP
语种英语
WOS研究方向Chemistry ; Engineering
WOS类目Chemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
WOS记录号WOS:000377388300015
引用统计
被引频次:3[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/8235
专题绿色化学催化团队
作者单位1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biobased Mat, Qingdao 266101, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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GB/T 7714
Liu, Xiaoran,Wang, Xicheng,Liu, Qiang,et al. A sustainable process for the production of 2-methyl-1,4-butanediol by hydrogenation of biomass-derived itaconic acid[J]. CATALYSIS TODAY,2016,274:88-93.
APA Liu, Xiaoran,Wang, Xicheng,Liu, Qiang,Xu, Guoqiang,Li, Xuemin,&Mu, Xindong.(2016).A sustainable process for the production of 2-methyl-1,4-butanediol by hydrogenation of biomass-derived itaconic acid.CATALYSIS TODAY,274,88-93.
MLA Liu, Xiaoran,et al."A sustainable process for the production of 2-methyl-1,4-butanediol by hydrogenation of biomass-derived itaconic acid".CATALYSIS TODAY 274(2016):88-93.
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