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High Conductive Two-Dimensional Covalent Organic Framework for Lithium Storage with Large Capacity
Yang, Hui1,3; Zhang, Shengliang2,3; Han, Liheng1; Zhang, Zhou1; Xue, Zheng1; Gao, Juan1,3; Li, Yongjun1; Huang, Changshui2; Yi, Yuanping1; Liu, Huibiao1; Li, Yuliang1
2016-03-02
Source PublicationACS APPLIED MATERIALS & INTERFACES
Volume8Issue:8Pages:5366-5375
AbstractA high conductive 2D COF polyporphyrin (TThPP) linked by 4-thiophenephenyl groups was synthesized through an in situ chemical oxidative polymerization on the surface of copper foil. The TThPP films were used as the anode of lithium-ion battery, which exhibited high specific capacities, excellent rate performances, and long cycle lives due to the alignment of 2D polyporphyrin nanosheets, and they (i) can highly efficiently adsorb Li atoms, (ii) have short-ended paths for the fast lithium ion diffusion, and (iii) open nanopores holding electrolyte. The reversible capacity is up to 666 mAh/g. This is the first example of an organic 2D COF for an anode of lithium-ion battery and represents an important step toward the use of COFs in the next-generation high-performance lithium ion battery.
SubtypeArticle
Keyword2d Cof Polyporphyrin High Conductive Lithium Storage High Capacity
WOS HeadingsScience & Technology ; Technology
DOI10.1021/acsami.5b12370
WOS KeywordION BATTERIES ; PHOTOPHYSICAL PROPERTIES ; PORPHYRIN ARRAYS ; HYDROGEN STORAGE ; THIN-FILMS ; PERFORMANCE ; CATHODE ; CRYSTALLINE ; POLYMERS ; ELECTRON
Indexed BySCI
Language英语
WOS Research AreaScience & Technology - Other Topics ; Materials Science
Funding OrganizationNational Basic Research 973 Program of China(2012CB932901) ; National Nature Science Foundation of China(51573191 ; Strategic Priority Research Program of the Chinese Academy of Sciences(XDB12010100) ; 21373235 ; 21290190)
WOS SubjectNanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS IDWOS:000371453600036
Citation statistics
Cited Times:68[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.qibebt.ac.cn/handle/337004/8059
Collection新型能源碳素材料团队
Affiliation1.Chinese Acad Sci, Inst Chem, CAS Key Lab Organ Solids, BNLMS, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China
3.Chinese Acad Sci, Grad Univ, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Yang, Hui,Zhang, Shengliang,Han, Liheng,et al. High Conductive Two-Dimensional Covalent Organic Framework for Lithium Storage with Large Capacity[J]. ACS APPLIED MATERIALS & INTERFACES,2016,8(8):5366-5375.
APA Yang, Hui.,Zhang, Shengliang.,Han, Liheng.,Zhang, Zhou.,Xue, Zheng.,...&Li, Yuliang.(2016).High Conductive Two-Dimensional Covalent Organic Framework for Lithium Storage with Large Capacity.ACS APPLIED MATERIALS & INTERFACES,8(8),5366-5375.
MLA Yang, Hui,et al."High Conductive Two-Dimensional Covalent Organic Framework for Lithium Storage with Large Capacity".ACS APPLIED MATERIALS & INTERFACES 8.8(2016):5366-5375.
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