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Transformative Evolution of Organolead Triiodide Perovskite Thin Films from Strong Room-Temperature Solid-Gas Interaction between HPbl(3)-CH3NH2 Precursor Pair
Pang, Shuping1; Zhou, Yuanyuan2; Wang, Zaiwei1; Yang, Mengjin3; Krause, Amanda R.2; Zhou, Zhongmin1; Zhu, Kai3; Padture, Nitin P.2; Cui, Guanglei1
2016-01-27
发表期刊JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷号138期号:3页码:750-753
摘要

We demonstrate the feasibility of a nonsalt-based precursor pair-inorganic HPbI3 solid and organic CH3NH2 gas-for the deposition of uniform CH3NH3PbI3 perovskite thin films. The strong room-temperature solidgas interaction between HPbI3 and CH3NH2 induces transformative evolution of ultrasmooth, full-coverage perovskite thin films at a rapid rate (in seconds) from nominally processed rough, partial-coverage HPbI3 thin films. The chemical origin of this behavior is elucidated via in situ experiments. Perovskite solar cells, fabricated using MAPbI(3) thin films thus deposited, deliver power conversion efficiencies up to 18.2%, attesting to the high quality of the perovskite thin films deposited using this transformative process.

文章类型Article
WOS标题词Science & Technology ; Physical Sciences
DOI10.1021/jacs.5b11824
关键词[WOS]SOLAR-CELLS ; HALIDE PEROVSKITES ; LIGHT ; STATE ; EXTRACTION ; EFFICIENT ; LAYERS
收录类别SCI
语种英语
WOS研究方向Chemistry
项目资助者International S&T Cooperation Program of China(2015DFG62670) ; Youth Innovation Promotion Association of CAS(2015167) ; Qingdao Key Lab of solar energy utilization and energy storage technology ; National Science Foundation(DMR-1305913 ; U.S. Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 program(DE-FOA-0000990 ; OIA-1538893) ; DE-AC36-08-GO28308)
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000369044400010
引用统计
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/8011
专题仿生与固态能源系统研究组
作者单位1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China
2.Brown Univ, Sch Engn, Providence, RI 02912 USA
3.Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA
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Pang, Shuping,Zhou, Yuanyuan,Wang, Zaiwei,et al. Transformative Evolution of Organolead Triiodide Perovskite Thin Films from Strong Room-Temperature Solid-Gas Interaction between HPbl(3)-CH3NH2 Precursor Pair[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2016,138(3):750-753.
APA Pang, Shuping.,Zhou, Yuanyuan.,Wang, Zaiwei.,Yang, Mengjin.,Krause, Amanda R..,...&Cui, Guanglei.(2016).Transformative Evolution of Organolead Triiodide Perovskite Thin Films from Strong Room-Temperature Solid-Gas Interaction between HPbl(3)-CH3NH2 Precursor Pair.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,138(3),750-753.
MLA Pang, Shuping,et al."Transformative Evolution of Organolead Triiodide Perovskite Thin Films from Strong Room-Temperature Solid-Gas Interaction between HPbl(3)-CH3NH2 Precursor Pair".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 138.3(2016):750-753.
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