| Transformative Evolution of Organolead Triiodide Perovskite Thin Films from Strong Room-Temperature Solid-Gas Interaction between HPbl(3)-CH3NH2 Precursor Pair | |
Pang, Shuping1 ; Zhou, Yuanyuan2; Wang, Zaiwei1; Yang, Mengjin3; Krause, Amanda R.2; Zhou, Zhongmin1; Zhu, Kai3; Padture, Nitin P.2; Cui, Guanglei1
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| 2016-01-27 | |
| Source Publication | JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
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| Volume | 138Issue:3Pages:750-753 |
| Abstract | We demonstrate the feasibility of a nonsalt-based precursor pair-inorganic HPbI3 solid and organic CH3NH2 gas-for the deposition of uniform CH3NH3PbI3 perovskite thin films. The strong room-temperature solidgas interaction between HPbI3 and CH3NH2 induces transformative evolution of ultrasmooth, full-coverage perovskite thin films at a rapid rate (in seconds) from nominally processed rough, partial-coverage HPbI3 thin films. The chemical origin of this behavior is elucidated via in situ experiments. Perovskite solar cells, fabricated using MAPbI(3) thin films thus deposited, deliver power conversion efficiencies up to 18.2%, attesting to the high quality of the perovskite thin films deposited using this transformative process. |
| Subtype | Article |
| WOS Headings | Science & Technology ; Physical Sciences |
| DOI | 10.1021/jacs.5b11824 |
| WOS Keyword | SOLAR-CELLS ; HALIDE PEROVSKITES ; LIGHT ; STATE ; EXTRACTION ; EFFICIENT ; LAYERS |
| Indexed By | SCI |
| Language | 英语 |
| WOS Research Area | Chemistry |
| Funding Organization | International S&T Cooperation Program of China(2015DFG62670) ; Youth Innovation Promotion Association of CAS(2015167) ; Qingdao Key Lab of solar energy utilization and energy storage technology ; National Science Foundation(DMR-1305913 ; U.S. Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 program(DE-FOA-0000990 ; OIA-1538893) ; DE-AC36-08-GO28308) |
| WOS Subject | Chemistry, Multidisciplinary |
| WOS ID | WOS:000369044400010 |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.qibebt.ac.cn/handle/337004/8011 |
| Collection | 仿生与固态能源系统研究组 |
| Affiliation | 1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China 2.Brown Univ, Sch Engn, Providence, RI 02912 USA 3.Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA |
| Recommended Citation GB/T 7714 | Pang, Shuping,Zhou, Yuanyuan,Wang, Zaiwei,et al. Transformative Evolution of Organolead Triiodide Perovskite Thin Films from Strong Room-Temperature Solid-Gas Interaction between HPbl(3)-CH3NH2 Precursor Pair[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2016,138(3):750-753. |
| APA | Pang, Shuping.,Zhou, Yuanyuan.,Wang, Zaiwei.,Yang, Mengjin.,Krause, Amanda R..,...&Cui, Guanglei.(2016).Transformative Evolution of Organolead Triiodide Perovskite Thin Films from Strong Room-Temperature Solid-Gas Interaction between HPbl(3)-CH3NH2 Precursor Pair.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,138(3),750-753. |
| MLA | Pang, Shuping,et al."Transformative Evolution of Organolead Triiodide Perovskite Thin Films from Strong Room-Temperature Solid-Gas Interaction between HPbl(3)-CH3NH2 Precursor Pair".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 138.3(2016):750-753. |
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| File Name/Size | DocType | Version | Access | License | ||
| Transformative Evolu（365KB） | 期刊论文 | 作者接受稿 | 开放获取 | CC BY-NC-SA | View Application Full Text | |
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