Hydrogen Peroxide-Assisted Sodium Carbonate Pretreatment for the Enhancement of Enzymatic Saccharification of Corn Stover | |
Gong, Wenbo1,2; Liu, Chao2; Mu, Xindong2; Du, Haishun2,3; Lv, Dong2; Li, Bin2; Han, Sheng1 | |
2015-12-01 | |
发表期刊 | ACS SUSTAINABLE CHEMISTRY & ENGINEERING |
卷号 | 3期号:12页码:3477-3485 |
摘要 | In this work, the effectiveness of hydrogen peroxide-assisted sodium carbonate (HSC) pretreatment of corn stover to produce fermentable sugars was investigated. It was found that the addition of H2O2 (a green oxidative agent) in Na2CO3 pretreatment could enhance the lignin removal and increase the hydrophilicity of the residual lignin, leading to the improved enzymatic digestibility and the yield of fermentable sugars. Also, results showed that lignin removal (in the range of 12-65%) was positively and linearly correlated with final total sugar yields. Post PFI refining could further improve the enzyme accessibility by increasing porosity of substrates. After HSC pretreatment (40 wt % Na2CO3 and 15 wt % H2O2 120 degrees C for 60 min) and enzymatic hydrolysis, the final total sugar yield could achieve 79%, which was about 10% higher in comparison with the conventional Na2CO3 pretreatment under the same conditions. HSC pretreatment will have less environmental impact and less barriers for large scale production. |
文章类型 | Article |
关键词 | Pretreatment Sodium Carbonate Hydrogen Peroxide Corn Stover Enzymatic Hydrolysis/saccharification |
WOS标题词 | Science & Technology ; Physical Sciences ; Technology |
DOI | 10.1021/acs.suschemeng.5b01278 |
关键词[WOS] | GREEN LIQUOR PRETREATMENT ; RICE STRAW ; ETHANOL-PRODUCTION ; HYDROLYSIS ; DIGESTIBILITY ; LIGNIN ; ALKALI ; CONVERSION ; HYDROXIDE |
收录类别 | SCI |
语种 | 英语 |
WOS研究方向 | Chemistry ; Engineering |
项目资助者 | National Natural Science Foundation of China(21306261 ; Subject of Plateau in Chemical Engineering and Technology of Shanghai (Flavor Technology and Engineering) ; Shandong Provincial Natural Science Foundation for Distinguished Young Scholar (China)(JQ201305) ; National High Technology Research and Development Program ("863" program) of China(2012AA022301) ; 31470609) |
WOS类目 | Chemistry, Multidisciplinary ; Engineering, Chemical |
WOS记录号 | WOS:000366153700055 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.qibebt.ac.cn/handle/337004/6815 |
专题 | 绿色化学催化研究组 |
作者单位 | 1.Shanghai Inst Technol, Sch Chem & Environm Engn, Shanghai 201418, Peoples R China 2.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, CAS Key Lab Biobased Mat, Qingdao 266101, Peoples R China 3.Tianjin Univ Sci & Technol, Coll Papermaking Sci & Technol, Tianjin Key Lab Pulp & Paper, Tianjin 300457, Peoples R China |
推荐引用方式 GB/T 7714 | Gong, Wenbo,Liu, Chao,Mu, Xindong,et al. Hydrogen Peroxide-Assisted Sodium Carbonate Pretreatment for the Enhancement of Enzymatic Saccharification of Corn Stover[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2015,3(12):3477-3485. |
APA | Gong, Wenbo.,Liu, Chao.,Mu, Xindong.,Du, Haishun.,Lv, Dong.,...&Han, Sheng.(2015).Hydrogen Peroxide-Assisted Sodium Carbonate Pretreatment for the Enhancement of Enzymatic Saccharification of Corn Stover.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,3(12),3477-3485. |
MLA | Gong, Wenbo,et al."Hydrogen Peroxide-Assisted Sodium Carbonate Pretreatment for the Enhancement of Enzymatic Saccharification of Corn Stover".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 3.12(2015):3477-3485. |
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