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Hydrogen Peroxide-Assisted Sodium Carbonate Pretreatment for the Enhancement of Enzymatic Saccharification of Corn Stover
Gong, Wenbo1,2; Liu, Chao2; Mu, Xindong2; Du, Haishun2,3; Lv, Dong2; Li, Bin2; Han, Sheng1
2015-12-01
发表期刊ACS SUSTAINABLE CHEMISTRY & ENGINEERING
卷号3期号:12页码:3477-3485
摘要In this work, the effectiveness of hydrogen peroxide-assisted sodium carbonate (HSC) pretreatment of corn stover to produce fermentable sugars was investigated. It was found that the addition of H2O2 (a green oxidative agent) in Na2CO3 pretreatment could enhance the lignin removal and increase the hydrophilicity of the residual lignin, leading to the improved enzymatic digestibility and the yield of fermentable sugars. Also, results showed that lignin removal (in the range of 12-65%) was positively and linearly correlated with final total sugar yields. Post PFI refining could further improve the enzyme accessibility by increasing porosity of substrates. After HSC pretreatment (40 wt % Na2CO3 and 15 wt % H2O2 120 degrees C for 60 min) and enzymatic hydrolysis, the final total sugar yield could achieve 79%, which was about 10% higher in comparison with the conventional Na2CO3 pretreatment under the same conditions. HSC pretreatment will have less environmental impact and less barriers for large scale production.
文章类型Article
关键词Pretreatment Sodium Carbonate Hydrogen Peroxide Corn Stover Enzymatic Hydrolysis/saccharification
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1021/acs.suschemeng.5b01278
关键词[WOS]GREEN LIQUOR PRETREATMENT ; RICE STRAW ; ETHANOL-PRODUCTION ; HYDROLYSIS ; DIGESTIBILITY ; LIGNIN ; ALKALI ; CONVERSION ; HYDROXIDE
收录类别SCI
语种英语
WOS研究方向Chemistry ; Engineering
项目资助者National Natural Science Foundation of China(21306261 ; Subject of Plateau in Chemical Engineering and Technology of Shanghai (Flavor Technology and Engineering) ; Shandong Provincial Natural Science Foundation for Distinguished Young Scholar (China)(JQ201305) ; National High Technology Research and Development Program ("863" program) of China(2012AA022301) ; 31470609)
WOS类目Chemistry, Multidisciplinary ; Engineering, Chemical
WOS记录号WOS:000366153700055
引用统计
被引频次:37[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/6815
专题绿色化学催化研究组
作者单位1.Shanghai Inst Technol, Sch Chem & Environm Engn, Shanghai 201418, Peoples R China
2.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, CAS Key Lab Biobased Mat, Qingdao 266101, Peoples R China
3.Tianjin Univ Sci & Technol, Coll Papermaking Sci & Technol, Tianjin Key Lab Pulp & Paper, Tianjin 300457, Peoples R China
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Gong, Wenbo,Liu, Chao,Mu, Xindong,et al. Hydrogen Peroxide-Assisted Sodium Carbonate Pretreatment for the Enhancement of Enzymatic Saccharification of Corn Stover[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2015,3(12):3477-3485.
APA Gong, Wenbo.,Liu, Chao.,Mu, Xindong.,Du, Haishun.,Lv, Dong.,...&Han, Sheng.(2015).Hydrogen Peroxide-Assisted Sodium Carbonate Pretreatment for the Enhancement of Enzymatic Saccharification of Corn Stover.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,3(12),3477-3485.
MLA Gong, Wenbo,et al."Hydrogen Peroxide-Assisted Sodium Carbonate Pretreatment for the Enhancement of Enzymatic Saccharification of Corn Stover".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 3.12(2015):3477-3485.
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