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Microstructures of Organometal Trihalide Perovskites for Solar Cells: Their Evolution from Solutions and Characterization
Zhou, Yuanyuan1; Game, Onkar S.1; Pang, Shuping2; Padture, Nitin P.1
2015-12-03
Source PublicationJOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume6Issue:23Pages:4827-4839
Abstract

The use of organometal trihalide perovskites (OTPs) in perovskite solar cells (PSCs) is revolutionizing the field of photovoltaics, which is being led by advances in solution processing of OTP thin films. First, we look at fundamental phenomena pertaining to nucleation/growth, coarsening, and microstructural evolution involved in the solution-processing of OTP thin films for PSCs from a materials-science perspective. Established scientific principles that govern some of these phenomena are invoked in the context of specific literature examples of solution-processed OTP thin films. Second, the nature and the unique characteristics of OTP thin-film microstructures themselves are discussed from a materials-science perspective. Finally, we discuss the challenges and opportunities in the characterization of OTP thin films for not only gaining a deep understanding of defects and microstructures but also elucidating classical and nonclassical phenomena pertaining to nucleation/growth, coarsening, and microstructural evolution in these films. The overall goal is to have deterministic control over the solution-processing of tailored OTP thin films with desired morphologies and microstructures.

SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1021/acs.jpclett.5b01843
WOS KeywordLEAD IODIDE PEROVSKITE ; ORGANIC-INORGANIC PEROVSKITES ; HIGH-EFFICIENCY ; THIN-FILMS ; ORGANOLEAD TRIHALIDE ; HALIDE PEROVSKITES ; CRYSTAL-GROWTH ; SEQUENTIAL DEPOSITION ; SINGLE-CRYSTALS ; HOLE-CONDUCTOR
Indexed BySCI
Language英语
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
Funding OrganizationNational Science Foundation(DMR-1305913 ; Chinese National Natural Science Foundation(51202266) ; OIA-1538893)
WOS SubjectChemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Atomic, Molecular & Chemical
WOS IDWOS:000366008500026
Citation statistics
Cited Times:143[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.qibebt.ac.cn/handle/337004/6814
Collection仿生能源与储能系统团队
Affiliation1.Brown Univ, Sch Engn, Providence, RI 02912 USA
2.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China
Recommended Citation
GB/T 7714
Zhou, Yuanyuan,Game, Onkar S.,Pang, Shuping,et al. Microstructures of Organometal Trihalide Perovskites for Solar Cells: Their Evolution from Solutions and Characterization[J]. JOURNAL OF PHYSICAL CHEMISTRY LETTERS,2015,6(23):4827-4839.
APA Zhou, Yuanyuan,Game, Onkar S.,Pang, Shuping,&Padture, Nitin P..(2015).Microstructures of Organometal Trihalide Perovskites for Solar Cells: Their Evolution from Solutions and Characterization.JOURNAL OF PHYSICAL CHEMISTRY LETTERS,6(23),4827-4839.
MLA Zhou, Yuanyuan,et al."Microstructures of Organometal Trihalide Perovskites for Solar Cells: Their Evolution from Solutions and Characterization".JOURNAL OF PHYSICAL CHEMISTRY LETTERS 6.23(2015):4827-4839.
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