TG-MS analysis and kinetic study for thermal decomposition of six representative components of municipal solid waste under steam atmosphere | |
Zhang, Jinzhi1,2; Chen, Tianju1; Wu, Jingli1; Wu, Jinhu1 | |
2015-09-01 | |
发表期刊 | WASTE MANAGEMENT |
卷号 | 43页码:152-161 |
摘要 | Thermal decomposition of six representative components of municipal solid waste (MSW, including lignin, printing paper, cotton, rubber, polyvinyl chloride (PVC) and cabbage) was investigated by thermogravimetric-mass spectroscopy (TG-MS) under steam atmosphere. Compared with TG and derivative thermogravimetric (DTG) curves under N-2 atmosphere, thermal decomposition of MSW components under steam atmosphere was divided into pyrolysis and gasification stages. In the pyrolysis stage, the shapes of TG and DTG curves under steam atmosphere were almost the same with those under N-2 atmosphere. In the gasification stage, the presence of steam led to a greater mass loss because of the steam partial oxidation of char residue. The evolution profiles of H-2, CH4, CO and CO2 were well consistent with DTG curves in terms of appearance of peaks and relevant stages in the whole temperature range, and the steam partial oxidation of char residue promoted the generation of more gas products in high temperature range. The multi-Gaussian distributed activation energy model (DAEM) was proved plausible to describe thermal decomposition behaviours of MSW components under steam atmosphere. (C) 2015 Elsevier Ltd. All rights reserved. |
文章类型 | Article |
关键词 | Pyrolysis Gasification Kinetic Analysis Steam Atmosphere Municipal Solid Waste (Msw) Thermogravimetric-mass Spectroscopy (Tg-ms) |
WOS标题词 | Science & Technology ; Technology ; Life Sciences & Biomedicine |
DOI | 10.1016/j.wasman.2015.05.024 |
关键词[WOS] | ACTIVATION-ENERGY MODEL ; DAEM-REACTION MODEL ; THERMOGRAVIMETRIC ANALYSIS ; PYROLYSIS KINETICS ; BIO-OIL ; BIOMASS ; LIGNIN ; PVC ; HEMICELLULOSE ; GASIFICATION |
收录类别 | SCI |
语种 | 英语 |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
WOS类目 | Engineering, Environmental ; Environmental Sciences |
WOS记录号 | WOS:000359873600017 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.qibebt.ac.cn/handle/337004/6502 |
专题 | 热化学转化研究组 |
作者单位 | 1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biofuels, Qingdao 266101, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Jinzhi,Chen, Tianju,Wu, Jingli,et al. TG-MS analysis and kinetic study for thermal decomposition of six representative components of municipal solid waste under steam atmosphere[J]. WASTE MANAGEMENT,2015,43:152-161. |
APA | Zhang, Jinzhi,Chen, Tianju,Wu, Jingli,&Wu, Jinhu.(2015).TG-MS analysis and kinetic study for thermal decomposition of six representative components of municipal solid waste under steam atmosphere.WASTE MANAGEMENT,43,152-161. |
MLA | Zhang, Jinzhi,et al."TG-MS analysis and kinetic study for thermal decomposition of six representative components of municipal solid waste under steam atmosphere".WASTE MANAGEMENT 43(2015):152-161. |
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