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Ni-Cu/ZnO-catalyzed Hydrogenolysis of Cellulose for the Production of 1,2-Alkanediols in Hot Compressed Water
Wang, Xicheng1,2; Wu, Feng1,3; Yao, Shengxi1; Jiang, Yijun1; Guan, Jing1; Mui, Xindong1
2012-05-05
发表期刊CHEMISTRY LETTERS
卷号41期号:5页码:476-478
摘要Ni-Cu/ZnO catalysts with varied Ni-to-Cu mole ratio were prepared by coprecipitation and evaluated for the hydrogenolysis of high-crystalline cellulose. Ni and Cu species exerted synergetic effects in dehydroxylation reaction and C-C bond breakage for the formation of 1,2-alkanediols. Ni-Cu/ZnO with Ni-to-Cu ratio of 2:3 is highly selective toward 1,2-alkanediols (72.5%) under hydrothermal conditions (518 K, 4 MPa H-2), which also exhibits excellent activity in the conversion of real biomass.
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
DOI10.1246/cl.2012.476
关键词[WOS]ETHYLENE-GLYCOL ; CONVERSION ; CHEMICALS ; GLYCEROL ; POLYOLS
收录类别SCI
语种英语
WOS研究方向Chemistry
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000304517600002
引用统计
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/6341
专题绿色化学催化研究组
作者单位1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biofuels, Qingdao 266101, Peoples R China
2.Grad Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Qingdao 266061, Peoples R China
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GB/T 7714
Wang, Xicheng,Wu, Feng,Yao, Shengxi,et al. Ni-Cu/ZnO-catalyzed Hydrogenolysis of Cellulose for the Production of 1,2-Alkanediols in Hot Compressed Water[J]. CHEMISTRY LETTERS,2012,41(5):476-478.
APA Wang, Xicheng,Wu, Feng,Yao, Shengxi,Jiang, Yijun,Guan, Jing,&Mui, Xindong.(2012).Ni-Cu/ZnO-catalyzed Hydrogenolysis of Cellulose for the Production of 1,2-Alkanediols in Hot Compressed Water.CHEMISTRY LETTERS,41(5),476-478.
MLA Wang, Xicheng,et al."Ni-Cu/ZnO-catalyzed Hydrogenolysis of Cellulose for the Production of 1,2-Alkanediols in Hot Compressed Water".CHEMISTRY LETTERS 41.5(2012):476-478.
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