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Infinite Metal-Carboxylate Nanotube Constructed Metal-Organic Frameworks and Gas Sorption Properties
Lv, Xiaoxia1,2; Tang, Sifu1; Li, Liangjun1,2; Cai, Jinjun1,2; Wang, Chao1,2; Xu, Xianrui1,2; Zhao, Xuebo1
2013-10-01
发表期刊EUROPEAN JOURNAL OF INORGANIC CHEMISTRY
卷号2013期号:29页码:5081-5085
摘要

Two isomorphic microporous metal-organic frameworks (MOFs), [Co2L(H2O)(2)]4.5H(2)O (1) and [Ni2L(H2O)(2)]3.5H(2)O (2), were synthesized by the reaction of an aminopolycarboxylate ligand (H4L) with Co and Ni hydroxides under hydrothermal conditions. The exquisite assembly of the carboxylate, imino groups, and metal ions resulted in a 1D special nanotube that could be used as a blueprint for the construction of MOFs. By joining the nanotubes with the V-shaped -CH2(C6H)(CH3)(3)CH2- spacer, a 3D framework with 1D triangular channels was formed. The two isostructural frameworks exhibited stability up to 350 degrees C. Gas sorption studies for N-2, H-2, CO2, and CH4 confirmed their permanent porosity.

文章类型Article
关键词Metal-organic Frameworks Nanotubes Adsorption Microporous Materials
WOS标题词Science & Technology ; Physical Sciences
DOI10.1002/ejic.201300714
关键词[WOS]SECONDARY BUILDING UNITS ; COORDINATION POLYMERS ; ADSORPTION PROPERTIES ; HYDROGEN STORAGE ; ACID ; PHOSPHONATES ; BLOCKS ; SERIES ; 2D
收录类别SCI
语种英语
WOS研究方向Chemistry
WOS类目Chemistry, Inorganic & Nuclear
WOS记录号WOS:000325151200010
引用统计
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/6019
专题储氢及新型纳孔材料团队(过去)
作者单位1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Shandong, Peoples R China
2.Univ Chinese Acad Sci, Beijing, Peoples R China
推荐引用方式
GB/T 7714
Lv, Xiaoxia,Tang, Sifu,Li, Liangjun,et al. Infinite Metal-Carboxylate Nanotube Constructed Metal-Organic Frameworks and Gas Sorption Properties[J]. EUROPEAN JOURNAL OF INORGANIC CHEMISTRY,2013,2013(29):5081-5085.
APA Lv, Xiaoxia.,Tang, Sifu.,Li, Liangjun.,Cai, Jinjun.,Wang, Chao.,...&Zhao, Xuebo.(2013).Infinite Metal-Carboxylate Nanotube Constructed Metal-Organic Frameworks and Gas Sorption Properties.EUROPEAN JOURNAL OF INORGANIC CHEMISTRY,2013(29),5081-5085.
MLA Lv, Xiaoxia,et al."Infinite Metal-Carboxylate Nanotube Constructed Metal-Organic Frameworks and Gas Sorption Properties".EUROPEAN JOURNAL OF INORGANIC CHEMISTRY 2013.29(2013):5081-5085.
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