KMS Qingdao Institute of Biomass Energy and Bioprocess Technology ,CAS
Performance Enhancement of Inverted Perovskite Solar Cells Based on Smooth and Compact PC61BM:SnO2 Electron Transport Layers | |
Wang, Yao1,2; Duan, Chenghao1; Li, Jiangsheng1; Han, Wei1; Zhao, Min1; Yao, Lili1; Wang, Yuanyuan1; Yan, Chao2; Jiu, Tonggang1 | |
2018-06-13 | |
发表期刊 | ACS APPLIED MATERIALS & INTERFACES |
ISSN | 1944-8244 |
卷号 | 10期号:23页码:20128-20135 |
摘要 | In this work, PC61BM:SnO2 electron transport layers (ETLs) were applied in inverted CH3NH3PbI3 perovskite solar cells, and a high power conversion efficiency of 19.7% could be obtained. It increased by 49.0% in comparison with the device based on PC61 BM-only ETL (13.2%). SnO2 nanocrystals with excellent dispersibility were employed here to fill the pinholes and cover the valleys of PC61BM layer, forming smooth and compact PC61BM:SnO2 layers. Simultaneously, the electron traps caused by deep-level native defects of SnO2 were reduced by PC61BM, proved by the space charge limited current analysis. Thus, PC61BM:SnO2 ETLs can inhibit both of the defects in PC61BM and SnO2 layers which contribute to the electron transport improvement and reduce the recombination loss. Moreover, the device stability based on the bilayer was significantly improved in comparison with the PC61 BM-only device and the performance of 85% could be maintained after 1 month. |
关键词 | SnO2 perovskite solar cell inverted structure electron traps device stability |
DOI | 10.1021/acsami.8b03444 |
关键词[WOS] | ORGANOMETAL HALIDE PEROVSKITES ; QUANTUM DOTS ; EFFICIENCY ; SNO2 ; HYSTERESIS ; GRAPHDIYNE ; STABILITY ; PCBM |
语种 | 英语 |
资助项目 | National Natural Science Foundation of China[51672288] ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Major Basic Research Program of Shandong Natural Science Foundation[ZR2017ZB0313] |
WOS研究方向 | Science & Technology - Other Topics ; Materials Science |
项目资助者 | National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Major Basic Research Program of Shandong Natural Science Foundation |
WOS类目 | Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
WOS记录号 | WOS:000435525100092 |
出版者 | AMER CHEMICAL SOC |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.qibebt.ac.cn/handle/337004/12487 |
专题 | 中国科学院青岛生物能源与过程研究所 |
通讯作者 | Jiu, Tonggang |
作者单位 | 1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Shandong, Peoples R China 2.Jiangsu Univ Sci & Technol, Coll Mat Sci & Engn, Zhenjiang 212003, Jiangsu, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Yao,Duan, Chenghao,Li, Jiangsheng,et al. Performance Enhancement of Inverted Perovskite Solar Cells Based on Smooth and Compact PC61BM:SnO2 Electron Transport Layers[J]. ACS APPLIED MATERIALS & INTERFACES,2018,10(23):20128-20135. |
APA | Wang, Yao.,Duan, Chenghao.,Li, Jiangsheng.,Han, Wei.,Zhao, Min.,...&Jiu, Tonggang.(2018).Performance Enhancement of Inverted Perovskite Solar Cells Based on Smooth and Compact PC61BM:SnO2 Electron Transport Layers.ACS APPLIED MATERIALS & INTERFACES,10(23),20128-20135. |
MLA | Wang, Yao,et al."Performance Enhancement of Inverted Perovskite Solar Cells Based on Smooth and Compact PC61BM:SnO2 Electron Transport Layers".ACS APPLIED MATERIALS & INTERFACES 10.23(2018):20128-20135. |
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