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Graphene oxide nanosheets/multi-walled carbon nanotubes hybrid as an excellent electrocatalytic material towards VO2+/VO2+ redox couples for vanadium redox flow batteries
Han, Pengxian1; Yue, Yanhua1; Liu, Zhihong1; Xu, Wei2; Zhang, Lixue1; Xu, Hongxia1; Dong, Shanmu1; Cui, Guanglei1
2011-11-01
发表期刊ENERGY & ENVIRONMENTAL SCIENCE
卷号4期号:11页码:4710-4717
摘要A graphene oxide nanosheets/multi-walled carbon nanotubes (GO/MWCNTs) hybrid with excellent electrocatalytic redox reversibility towards VO2+/VO2+ redox couples for vanadium redox flow batteries (VRFB) has been prepared by an electrostatic spray technique after efficient ultrasonic treatment. The structures and electrochemical properties of GO/MWCNTs are investigated by transmission electron microscopy, scanning electron microscopy, X-ray diffraction, X-ray photoelectron spectroscopy, Raman spectroscopy and cyclic voltammetry. GO/MWCNTs are shown to be cross-linked and form an electrocatalytic hybrid with an effective mixed conducting network, leading to efficiently fast ion and electron transport characteristics. Compared with the pure GO nanosheets and MWCNTs, GO/MWCNTs deliver a much better electrocatalytic redox reversibility towards the positive VO2+/VO2+ couple, especially for the reduction from VO2+ to VO2+. The excellent experimental results demonstrate that the newly developed hybrid material holds great promise in the application of VRFB.
文章类型Article
学科领域仿生能源系统
WOS标题词Science & Technology ; Physical Sciences ; Technology ; Life Sciences & Biomedicine
DOI10.1039/c1ee01776d
关键词[WOS]GRAPHITE ELECTRODE MATERIALS ; CHEMICAL MODIFICATION ; FILMS ; CELL ; IMPEDANCE ; STORAGE ; SHEETS ; TRANSPARENT ; FELT
收录类别SCI
语种英语
WOS研究方向Chemistry ; Energy & Fuels ; Engineering ; Environmental Sciences & Ecology
WOS类目Chemistry, Multidisciplinary ; Energy & Fuels ; Engineering, Chemical ; Environmental Sciences
WOS记录号WOS:000296248100037
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被引频次:158[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/1166
专题仿生能源与储能系统团队
作者单位1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China
2.Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China
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Han, Pengxian,Yue, Yanhua,Liu, Zhihong,et al. Graphene oxide nanosheets/multi-walled carbon nanotubes hybrid as an excellent electrocatalytic material towards VO2+/VO2+ redox couples for vanadium redox flow batteries[J]. ENERGY & ENVIRONMENTAL SCIENCE,2011,4(11):4710-4717.
APA Han, Pengxian.,Yue, Yanhua.,Liu, Zhihong.,Xu, Wei.,Zhang, Lixue.,...&Cui, Guanglei.(2011).Graphene oxide nanosheets/multi-walled carbon nanotubes hybrid as an excellent electrocatalytic material towards VO2+/VO2+ redox couples for vanadium redox flow batteries.ENERGY & ENVIRONMENTAL SCIENCE,4(11),4710-4717.
MLA Han, Pengxian,et al."Graphene oxide nanosheets/multi-walled carbon nanotubes hybrid as an excellent electrocatalytic material towards VO2+/VO2+ redox couples for vanadium redox flow batteries".ENERGY & ENVIRONMENTAL SCIENCE 4.11(2011):4710-4717.
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