KMS Qingdao Institute of Biomass Energy and Bioprocess Technology ,CAS
One-step reduction synthesis of Ag/Ag3PO4/AgBr sub-micron composites for enhanced visible photocatalytic degradation of methyl orange | |
Yu, Zhuanni1; Xu, Mengmeng2; Wang, Qiang1; Sun, Xiaowei1; Lan, Jing1 | |
2018-08-01 | |
发表期刊 | MATERIALS RESEARCH BULLETIN
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ISSN | 0025-5408 |
卷号 | 104页码:149-154 |
摘要 | An efficient semiconductor composite, silver/silver orthophosphate/silver bromide, was successfully synthesized by a facile one-step reduction and ion exchange process. Its crystal structure, morphology, optical property, surface element composition were characterized by X-ray diffraction, scanning electron microscopy, ultraviolet-visible diffuse reflectance spectrometer and X-ray photoelectron spectrometer. The effects of composite proportion and synthesis duration on performances of as-prepared photocatalysts were investigated, and the results showed that Br/P molar ratio of 3 and the synthesis duration of 4 h were the optimum conditions. The radical scavenging experiments indicated that the hole and superoxide radical were the main active species in this reaction system. The Ag/Ag3PO4/AgBr-3 presented excellent stability and recyclability, maintaining 92% of degradation efficiency after 5 cycles. The good photocatalysis performance could be attributed to the formation of the heterojunction between Ag and Ag3PO4/AgBr. |
文章类型 | Article |
关键词 | Ag3po4/agbr One-step Reduction Photocatalytic Mechanism Stability |
WOS标题词 | Science & Technology ; Technology |
DOI | 10.1016/j.materresbull.2018.04.003 |
关键词[WOS] | LIGHT IRRADIATION ; AG3PO4 ; SEMICONDUCTOR ; WATER ; STABILITY ; MECHANISM ; HYBRIDS ; RHB ; AG |
收录类别 | SCI |
语种 | 英语 |
WOS研究方向 | Materials Science |
项目资助者 | National Natural Science Foundation(21407086) ; Doctor Fund of Qingdao Agricultural University(63311330 ; 63311203) |
WOS类目 | Materials Science, Multidisciplinary |
WOS记录号 | WOS:000432769900024 |
出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.qibebt.ac.cn/handle/337004/11442 |
专题 | 中国科学院青岛生物能源与过程研究所 |
通讯作者 | Lan, Jing |
作者单位 | 1.Qingdao Agr Univ, Coll Chem & Pharmaceut Sci, Qingdao 266109, Peoples R China 2.Chinese Acad Sci, Qingdao Inst Biomass Energy & Bioproc Technol, CAS Key Lab Biobased Mat, Qingdao 266101, Peoples R China |
推荐引用方式 GB/T 7714 | Yu, Zhuanni,Xu, Mengmeng,Wang, Qiang,et al. One-step reduction synthesis of Ag/Ag3PO4/AgBr sub-micron composites for enhanced visible photocatalytic degradation of methyl orange[J]. MATERIALS RESEARCH BULLETIN,2018,104:149-154. |
APA | Yu, Zhuanni,Xu, Mengmeng,Wang, Qiang,Sun, Xiaowei,&Lan, Jing.(2018).One-step reduction synthesis of Ag/Ag3PO4/AgBr sub-micron composites for enhanced visible photocatalytic degradation of methyl orange.MATERIALS RESEARCH BULLETIN,104,149-154. |
MLA | Yu, Zhuanni,et al."One-step reduction synthesis of Ag/Ag3PO4/AgBr sub-micron composites for enhanced visible photocatalytic degradation of methyl orange".MATERIALS RESEARCH BULLETIN 104(2018):149-154. |
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