QIBEBT-IR
One-step reduction synthesis of Ag/Ag3PO4/AgBr sub-micron composites for enhanced visible photocatalytic degradation of methyl orange
Yu, Zhuanni1; Xu, Mengmeng2; Wang, Qiang1; Sun, Xiaowei1; Lan, Jing1
2018-08-01
发表期刊MATERIALS RESEARCH BULLETIN
ISSN0025-5408
卷号104页码:149-154
摘要An efficient semiconductor composite, silver/silver orthophosphate/silver bromide, was successfully synthesized by a facile one-step reduction and ion exchange process. Its crystal structure, morphology, optical property, surface element composition were characterized by X-ray diffraction, scanning electron microscopy, ultraviolet-visible diffuse reflectance spectrometer and X-ray photoelectron spectrometer. The effects of composite proportion and synthesis duration on performances of as-prepared photocatalysts were investigated, and the results showed that Br/P molar ratio of 3 and the synthesis duration of 4 h were the optimum conditions. The radical scavenging experiments indicated that the hole and superoxide radical were the main active species in this reaction system. The Ag/Ag3PO4/AgBr-3 presented excellent stability and recyclability, maintaining 92% of degradation efficiency after 5 cycles. The good photocatalysis performance could be attributed to the formation of the heterojunction between Ag and Ag3PO4/AgBr.
文章类型Article
关键词Ag3po4/agbr One-step Reduction Photocatalytic Mechanism Stability
WOS标题词Science & Technology ; Technology
DOI10.1016/j.materresbull.2018.04.003
关键词[WOS]LIGHT IRRADIATION ; AG3PO4 ; SEMICONDUCTOR ; WATER ; STABILITY ; MECHANISM ; HYBRIDS ; RHB ; AG
收录类别SCI
语种英语
WOS研究方向Materials Science
项目资助者National Natural Science Foundation(21407086) ; Doctor Fund of Qingdao Agricultural University(63311330 ; 63311203)
WOS类目Materials Science, Multidisciplinary
WOS记录号WOS:000432769900024
出版者PERGAMON-ELSEVIER SCIENCE LTD
引用统计
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/11442
专题中国科学院青岛生物能源与过程研究所
通讯作者Lan, Jing
作者单位1.Qingdao Agr Univ, Coll Chem & Pharmaceut Sci, Qingdao 266109, Peoples R China
2.Chinese Acad Sci, Qingdao Inst Biomass Energy & Bioproc Technol, CAS Key Lab Biobased Mat, Qingdao 266101, Peoples R China
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Yu, Zhuanni,Xu, Mengmeng,Wang, Qiang,et al. One-step reduction synthesis of Ag/Ag3PO4/AgBr sub-micron composites for enhanced visible photocatalytic degradation of methyl orange[J]. MATERIALS RESEARCH BULLETIN,2018,104:149-154.
APA Yu, Zhuanni,Xu, Mengmeng,Wang, Qiang,Sun, Xiaowei,&Lan, Jing.(2018).One-step reduction synthesis of Ag/Ag3PO4/AgBr sub-micron composites for enhanced visible photocatalytic degradation of methyl orange.MATERIALS RESEARCH BULLETIN,104,149-154.
MLA Yu, Zhuanni,et al."One-step reduction synthesis of Ag/Ag3PO4/AgBr sub-micron composites for enhanced visible photocatalytic degradation of methyl orange".MATERIALS RESEARCH BULLETIN 104(2018):149-154.
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