QIBEBT-IR
Electric-Field-Directed Parallel Alignment Architecting 3D Lithium-Ion Pathways within Solid Composite Electrolyte
Liu, Xueqing1,2; Peng, Sha1,2; Gao, Shuyu1; Cao, Yuancheng1; You, Qingliang2; Zhou, Liyong2; Jin, Yongcheng3; Liu, Zhihong1; Liu, Jiyan1,2
2018-05-09
Source PublicationACS APPLIED MATERIALS & INTERFACES
ISSN1944-8244
Volume10Issue:18Pages:15691-15696
AbstractIt is of great significance to seek high-performance solid electrolytes via a facile chemistry and simple process for meeting the requirements of solid batteries. Previous reports revealed that ion conducting pathways within ceramic-polymer composite electrolytes mainly occur at ceramic particles and the ceramic-polymer interface. Herein, one facile strategy toward ceramic particles' alignment and assembly induced by an external alternating-current (AC) electric field is presented. It was manifested by an in situ optical microscope that Li1.3Al0.3Ti1.7(PO4)(3) particles and poly(ethylene glycol) diacrylate in poly(dimethylsiloxane) (LATP@PEGDA@PDMS) assembled into three-dimensional connected networks on applying an external AC electric field. Scanning electron microscopy revealed that the ceramic LATP particles aligned into a necklacelike assembly. Electrochemical impedance spectroscopy confirmed that the ionic conductivity of this necklacelike alignment was significantly enhanced compared to that of the random one. It was demonstrated that this facile strategy of applying an AC electric field can be a very effective approach for architecting three-dimensional lithium-ion conductive networks within solid composite electrolyte.
SubtypeArticle
KeywordSolid Composite Electrolyte Electric Field Ceramic Particles Alignment Ionic Conductivity
WOS HeadingsScience & Technology ; Technology
DOI10.1021/acsami.8b01631
WOS KeywordPOLYMER ELECTROLYTES ; POLYETHYLENE OXIDE ; BATTERIES ; CONDUCTIVITY ; NANOPARTICLES ; TRANSPORT ; ENHANCEMENT ; FILMS ; GLASS
Indexed BySCI
Language英语
WOS Research AreaScience & Technology - Other Topics ; Materials Science
Funding OrganizationNational Key Research and Development (R&D) Program of China(2016YFB0401505) ; "Chutian Scholar Program" of Hubei province
WOS SubjectNanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS IDWOS:000432205800041
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:25[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.qibebt.ac.cn/handle/337004/11406
Collection中国科学院青岛生物能源与过程研究所
Corresponding AuthorLiu, Zhihong; Liu, Jiyan
Affiliation1.Jianghan Univ, Minist Educ, Key Lab Optoelect Chem Mat & Devices, Wuhan 430056, Hubei, Peoples R China
2.Jianghan Univ, Flexible Display Mat & Technol Coinnovat Ctr Hube, Wuhan 430056, Hubei, Peoples R China
3.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China
Recommended Citation
GB/T 7714
Liu, Xueqing,Peng, Sha,Gao, Shuyu,et al. Electric-Field-Directed Parallel Alignment Architecting 3D Lithium-Ion Pathways within Solid Composite Electrolyte[J]. ACS APPLIED MATERIALS & INTERFACES,2018,10(18):15691-15696.
APA Liu, Xueqing.,Peng, Sha.,Gao, Shuyu.,Cao, Yuancheng.,You, Qingliang.,...&Liu, Jiyan.(2018).Electric-Field-Directed Parallel Alignment Architecting 3D Lithium-Ion Pathways within Solid Composite Electrolyte.ACS APPLIED MATERIALS & INTERFACES,10(18),15691-15696.
MLA Liu, Xueqing,et al."Electric-Field-Directed Parallel Alignment Architecting 3D Lithium-Ion Pathways within Solid Composite Electrolyte".ACS APPLIED MATERIALS & INTERFACES 10.18(2018):15691-15696.
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