QIBEBT-IR
Electric-Field-Directed Parallel Alignment Architecting 3D Lithium-Ion Pathways within Solid Composite Electrolyte
Liu, Xueqing1,2; Peng, Sha1,2; Gao, Shuyu1; Cao, Yuancheng1; You, Qingliang2; Zhou, Liyong2; Jin, Yongcheng3; Liu, Zhihong1; Liu, Jiyan1,2
2018-05-09
发表期刊ACS APPLIED MATERIALS & INTERFACES
ISSN1944-8244
卷号10期号:18页码:15691-15696
摘要It is of great significance to seek high-performance solid electrolytes via a facile chemistry and simple process for meeting the requirements of solid batteries. Previous reports revealed that ion conducting pathways within ceramic-polymer composite electrolytes mainly occur at ceramic particles and the ceramic-polymer interface. Herein, one facile strategy toward ceramic particles' alignment and assembly induced by an external alternating-current (AC) electric field is presented. It was manifested by an in situ optical microscope that Li1.3Al0.3Ti1.7(PO4)(3) particles and poly(ethylene glycol) diacrylate in poly(dimethylsiloxane) (LATP@PEGDA@PDMS) assembled into three-dimensional connected networks on applying an external AC electric field. Scanning electron microscopy revealed that the ceramic LATP particles aligned into a necklacelike assembly. Electrochemical impedance spectroscopy confirmed that the ionic conductivity of this necklacelike alignment was significantly enhanced compared to that of the random one. It was demonstrated that this facile strategy of applying an AC electric field can be a very effective approach for architecting three-dimensional lithium-ion conductive networks within solid composite electrolyte.
文章类型Article
关键词Solid Composite Electrolyte Electric Field Ceramic Particles Alignment Ionic Conductivity
WOS标题词Science & Technology ; Technology
DOI10.1021/acsami.8b01631
关键词[WOS]POLYMER ELECTROLYTES ; POLYETHYLENE OXIDE ; BATTERIES ; CONDUCTIVITY ; NANOPARTICLES ; TRANSPORT ; ENHANCEMENT ; FILMS ; GLASS
收录类别SCI
语种英语
WOS研究方向Science & Technology - Other Topics ; Materials Science
项目资助者National Key Research and Development (R&D) Program of China(2016YFB0401505) ; "Chutian Scholar Program" of Hubei province
WOS类目Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号WOS:000432205800041
出版者AMER CHEMICAL SOC
引用统计
文献类型期刊论文
条目标识符http://ir.qibebt.ac.cn/handle/337004/11406
专题中国科学院青岛生物能源与过程研究所
通讯作者Liu, Zhihong; Liu, Jiyan
作者单位1.Jianghan Univ, Minist Educ, Key Lab Optoelect Chem Mat & Devices, Wuhan 430056, Hubei, Peoples R China
2.Jianghan Univ, Flexible Display Mat & Technol Coinnovat Ctr Hube, Wuhan 430056, Hubei, Peoples R China
3.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China
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Liu, Xueqing,Peng, Sha,Gao, Shuyu,et al. Electric-Field-Directed Parallel Alignment Architecting 3D Lithium-Ion Pathways within Solid Composite Electrolyte[J]. ACS APPLIED MATERIALS & INTERFACES,2018,10(18):15691-15696.
APA Liu, Xueqing.,Peng, Sha.,Gao, Shuyu.,Cao, Yuancheng.,You, Qingliang.,...&Liu, Jiyan.(2018).Electric-Field-Directed Parallel Alignment Architecting 3D Lithium-Ion Pathways within Solid Composite Electrolyte.ACS APPLIED MATERIALS & INTERFACES,10(18),15691-15696.
MLA Liu, Xueqing,et al."Electric-Field-Directed Parallel Alignment Architecting 3D Lithium-Ion Pathways within Solid Composite Electrolyte".ACS APPLIED MATERIALS & INTERFACES 10.18(2018):15691-15696.
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