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Enhanced Rate Performance of Al-Doped Li-Rich Layered Cathode Material via Nucleation and Post-solvothermal Method
Yang, Wenchao1; Xie, Yu1; Jiang, Jicheng1,2; Sun, Deye1; Ma, Xiaodi1; Lan, Zhenggang1; Jin, Yongcheng1
2018-04-01
Source PublicationACS SUSTAINABLE CHEMISTRY & ENGINEERING
ISSN2168-0485
Volume6Issue:4Pages:4625-4632
AbstractAl-doped layered cathode materials Li1.5-xAlxMn0.675Ni0.1675Co0.1675O2 have been successfully synthesized via a rapid nucleation and post-solvothermal method. The surface morphology and crystal structures of Al-doped Li-rich materials are investigated via scanning electron microscopy, X-ray diffraction, Raman spectra, and X-ray photoelectron spectroscopy. After optimization, the Li1.45Al0.05Mn0.675Ni0.1675Co0.1675O2 (Al = 0.05) sample showed excellent electrochemical performance, and the discharge capacities are 323.7 and 120 mAh g(-1) at a rate of 0.1 and 20 C,respectively. These improvements, based on electrochemical performance evaluation and density functional theory calculations, might be ascribed to the increased electron conductivity of layered Li-rich material via Al3+ ions doped into a crystal structure.
SubtypeArticle
KeywordLithium Ion Batteries Li-rich Material Al Doping High Rate Performance Density Functional Theory
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1021/acssuschemeng.7b03634
WOS KeywordLITHIUM-ION BATTERIES ; HIGH-CAPACITY ; ELECTROCHEMICAL PERFORMANCE ; CYCLING STABILITY ; COPRECIPITATION STRATEGY ; RECHARGEABLE BATTERIES ; COMPOSITE CATHODES ; RATE CAPABILITY ; SPINEL PHASE ; VOLTAGE FADE
Indexed BySCI
Language英语
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Engineering
Funding OrganizationChinese Academy of Sciences ; (YZ201641)
WOS SubjectChemistry, Multidisciplinary ; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY ; Engineering, Chemical
WOS IDWOS:000429285800022
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:5[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.qibebt.ac.cn/handle/337004/10820
Collection仿真与模拟团队
先进界面技术团队
Corresponding AuthorLan, Zhenggang; Jin, Yongcheng
Affiliation1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao Ind Energy Storage Technol Inst, Qingdao 266101, Peoples R China
2.Univ Chinese Acad Sci, 19A Yuquanlu Rd, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Yang, Wenchao,Xie, Yu,Jiang, Jicheng,et al. Enhanced Rate Performance of Al-Doped Li-Rich Layered Cathode Material via Nucleation and Post-solvothermal Method[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2018,6(4):4625-4632.
APA Yang, Wenchao.,Xie, Yu.,Jiang, Jicheng.,Sun, Deye.,Ma, Xiaodi.,...&Jin, Yongcheng.(2018).Enhanced Rate Performance of Al-Doped Li-Rich Layered Cathode Material via Nucleation and Post-solvothermal Method.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,6(4),4625-4632.
MLA Yang, Wenchao,et al."Enhanced Rate Performance of Al-Doped Li-Rich Layered Cathode Material via Nucleation and Post-solvothermal Method".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 6.4(2018):4625-4632.
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